A Solution‐Mediated Pathway for the Growth of the Solid Electrolyte Interphase in Lithium‐Ion Batteries (Adv. Energy Mater. 14/2023). Issue 14 (13th April 2023)

• Record Type: Journal Article
• Authors: Esmaeilpour, Meysam; Jana, Saibal; Li, Hongjiao; Soleymanibrojeni, Mohammad; Wenzel, Wolfgang
• Is Part Of: Advanced energy materials. Volume 13:Issue 14(2023)
• Page Start: n/a
• Page End: n/a
• Publication Date: 2023-04-13
• Subjects: interfacial reactivity -- kinetic Monte Carlo simulation -- lithium‐ion batteries -- machine learning -- multiscale modeling -- solid electrolyte interphase; Energy harvesting -- Materials -- Periodicals; Energy conversion -- Materials -- Periodicals; Energy storage -- Materials -- Periodicals; Photovoltaics -- Periodicals; Fuel cells -- Periodicals; Thermoelectric materials -- Periodicals; 621.31
• DOI: 10.1002/aenm.202370055
• Languages: English
• ISSNs: 1614-6832

Abstract

Abstract : Solid Electrolyte Interphase In article number 2203966, Wolfgang Wenzel and co‐workers use a mesoscale simulation approach to comprehensively characterize the growth and composition of the solid electrolyte interphase (SEI) based on a chemistry‐specific reaction network. They find that the organic SEI forms and grows in a solution‐mediated pathway by the aggregation of SEI precursors far away from the surface via a nucleation process, which has consequences for long‐term battery operation.