Thermal reshaping as a route for reuse of end-of-life glass fibre-reinforced acrylic composites. (15th May 2023)

• Record Type: Journal Article
• Authors: Obande, Winifred; Stankovic, Danijela; Bajpai, Ankur; Devine, Machar; Wurzer, Christian; Lykkeberg, Anna; Garden, Jennifer A.; Ó Brádaigh, Conchúr M.; Ray, Dipa
• Is Part Of: Composites. Number 257(2023)
• Publication Date: 2023-05-15
• Subjects: Composite materials -- Periodicals; Materials science -- Periodicals; Composite materials; Periodicals; Electronic journals; 620.118
• DOI: 10.1016/j.compositesb.2023.110662
• Languages: English
• ISSNs: 1359-8368

Abstract

Abstract: Thermal reshaping has been employed to simulate the end-of-life reuse of liquid-resin-infused thermoplastic acrylic composite laminates, and the associated effects on matrix-dominated mechanical performance and microstructure have been studied. L-shaped laminates were infused at room temperature and subjected to 1 or 4 hot-press flattening cycles (25 min at 120 °C; 11 bar). Compared to the original references, up to 13% higher transverse flexural strengths were measured for the reprocessed laminates. Such a scheme may be readily implemented for high-value reuse without sacrificing fibre length scales, and with minimal cumulative mass loss over successive reheating cycles (10 cycles: 2% and 15 cycles: 2.6%). This study provides important insights to foster a greater understanding of the performance limits of hot-press reprocessing to inform the practical reuse and re-application of sustainable composites in a circular economy. Graphical abstract: Image 1 Highlights: Thermal reshaping was demonstrated for high-value, end-of-life composite reuse. High fibre length-scale retention attainable in thermoplastic acrylic composites. L-shaped laminates were flattened in a hot platen press (120 °C; 11 bar) and tested. Transverse flexural strength increases by 13% after one reprocessing cycle. Up to 15 cycles may be applied with low oxidation-induced mass losses (<3%).