Dry Deposition of Reactive Nitrogen From Satellite Observations of Ammonia and Nitrogen Dioxide Over North America. Issue 2 (25th January 2018)

• Record Type: Journal Article
• Authors: Kharol, S. K.; Shephard, M. W.; McLinden, C. A.; Zhang, L.; Sioris, C. E.; O'Brien, J. M.; Vet, R.; Cady‐Pereira, K. E.; Hare, E.; Siemons, J.; Krotkov, N. A.
• Is Part Of: Geophysical research letters. Volume 45:Issue 2(2018)
• Page Start: 1157
• Page End: 1166
• Publication Date: 2018-01-25
• Subjects: dissolved organic carbon -- average carbon oxidation state -- GEOS‐Chem; Geophysics -- Periodicals; Planets -- Periodicals; Lunar geology -- Periodicals; 550
• DOI: 10.1002/2017GL075832
• Languages: English
• ISSNs: 0094-8276

Abstract

Abstract: Reactive nitrogen (Nr ) is an essential nutrient to plants and a limiting element for growth in many ecosystems, but it can have harmful effects on ecosystems when in excess. Satellite‐derived surface observations are used together with a dry deposition model to estimate the dry deposition flux of the most abundant short‐lived nitrogen species, NH3 and NO2, over North America during the 2013 warm season. These fluxes demonstrate that the NH3 contribution dominates over NO2 for most regions (comprising ~85% of their sum in Canada and ~65% in the U.S.), with some regional exceptions (e.g. Alberta and northeastern U.S.). Nationwide, ~1.35 Tg of N from these species were dry deposited in the contiguous U.S., more than double the ~0.61 Tg in Canada (excluding territories) over this period. Forest fires are shown to be the major contributor of dry deposition of Nr from NH3 in northern latitudes, leading to deposition fluxes 2–3 times greater than from expected amounts without fires. Key Points: First use of satellite observations to estimate the dry deposition of reactive nitrogen (Nr ) from ammonia (NH3 ) Satellite estimates of NH3 and NO2 dry deposition indicate that the NH3 dominates over most regions across the North America during the 2013 warm season Locations at northern latitudes affected by forest fires tend to have 2–3 times more dry deposition of ammonia relative to the local background