Signatures of Topological Surface State and Unconventional Magnetotransport Properties in Elemental Ruthenium. Issue 3 (15th January 2023)

• Record Type: Journal Article
• Authors: Singha, Ratnadwip; Sarkar, Shuvam; Ghosh, Arup; Roy, Shubhankar; Barman, Sajal; Balal, Mohammad; Barman, Sudipta Roy; Mandal, Prabhat
• Is Part Of: Advanced quantum technologies. Volume 6:Issue 3(2023)
• Page Start: n/a
• Page End: n/a
• Publication Date: 2023-01-15
• Subjects: angle resolved photoemission spectroscopy -- Dirac surface state -- magnetotransport properties -- planar Hall effect -- topological material; Quantum theory -- Periodicals; Quantum computing -- Periodicals; Quantum chemistry -- Periodicals; Quantum electronics -- Periodicals; 537.5
• DOI: 10.1002/qute.202200116
• Languages: English
• ISSNs: 2511-9044

Abstract

Abstract: In recent years, the pursuit of new topological materials has created a vast and ever growing catalogue of compounds. However, the example of elemental topological metals is still rather limited. So far, the non‐trivial topological states have been probed in only a handful of elements and that too rarely in a transition metal. By combining the angle‐resolved photoemission spectroscopy (ARPES) and magnetotransport measurements, here, ruthenium (Ru) is experimentally confirmed to be a topological metal, validating a recent theoretical prediction. The ARPES data for Ru(0001) provide evidence of the topological surface state related to the bulk Dirac node. Ru also exhibits a prominent planar Hall effect, thus further indicating its Dirac semimetallic nature. Large electron and hole mobilities are estimated, which are comparable to several topological semimetals. The non‐trivial nature of electronic band of Ru is also supported by the large non‐saturating transverse magnetoresistance. Abstract : From the theoretical calculations, elemental ruthenium is predicted to be the first 4 d transition metal with a topological Dirac state. The Dirac surface state is experimentally observed using angle‐resolved photo‐emission spectroscopy. The non‐trivial topological band structure also produces unconventional electronic transport properties including a robust planar Hall effect.