Lattice defects related magnetic and magnetocapacitance properties of multiferroic BaFe10.2Sc1.8O19 epitaxial thin films. (15th March 2022)

• Record Type: Journal Article
• Authors: Xu, Sichen; Zhu, Qishan; Liang, Guoqing; Zhang, Jianmin; Wang, Han; Wang, Haiyan; Zhao, Run; You, Lu; Su, Xiaodong; Tang, Rujun
• Is Part Of: Scripta materialia. Number 210(2022)
• Publication Date: 2022-03-15
• Subjects: Hexaferrite -- Thin film -- Lattice defects -- Magnetic -- Magnetocapacitance; Materials -- Periodicals; Metallurgy -- Periodicals; Metalen; Legeringen; Materiaalkunde; Metals, metalworking and machinery industries; Metals; Electronic journals; 620.11
• DOI: 10.1016/j.scriptamat.2021.114466
• Languages: English
• ISSNs: 1359-6462

Abstract

Abstract: Without changing the crystalline structure of BaFe10.2 Sc1.8 O19 (BFSO) epitaxial thin film, significant modulation of its saturation magnetization (from 75 to 180 emu/cc), magnetic anisotropy field (from 3590 to 1434 Oe) and multiferroic ordering temperature (from 207 to 306 K) can be realized with different densities of lattice defects (DLD). A defects-related effective magnetic field Heff is defined. Heff reduces obviously with increasing annealing temperature TA, agreeing well with the reduced DLD. The defects-related magnetic ordering of BFSO films is further verified in the magnetocapacitance devices. The magnetocapacitance for 1000 °C annealed film is more than 5 times larger than that of as-deposited film. This can be explained by the ultra-sensitive of non-collinear conical magnetic structure and spin-phonon coupling in BFSO to the DLD related local lattice structure. The above findings enable better understanding and usage of lattice defects on regulating the physical properties of multiferroic hexaferrite devices. Graphical abstract: Image, graphical abstract