SOFC Stack Operation: Effects of Electrode-Interconnect Contacts. (2nd June 2015)

• Record Type: Journal Article
• Authors: Minh, Nguyen; Budur, Abhijith; Dogan, Fatih
• Is Part Of: ECS transactions. Volume 68:Number 1(2015)
• Page Start: 2273
• Page End: 2278
• Publication Date: 2015-06-02
• Subjects: Electrochemistry -- Periodicals; Electrochemistry; Periodicals; Electronic journals; Electronic journal; 541.37
• DOI: 10.1149/06801.2273ecst
• Languages: English
• ISSNs: 1938-5862

Abstract

Abstract : Planar SOFC multi-cell stacks incorporating metallic interconnects generally exhibit average cell performance lower than that observed for out-of-stack cells under similar conditions. It has been suggested that electrode-interconnect, especially cathode-interconnect, contacts (and their ohmic resistances) are the main cause for this observed difference. In addition, cathode-interconnect contacts can evolve in long-term operation, resulting in stack performance reduction/degradation with time. Experiments using current interruption, AC electrochemical impedance and other characterization techniques have been conducted on single-cell stacks and button cells in contact with interconnect materials. The data obtained to date confirmed the hypothesis that contact ohmic resistance significantly contributes to stack performance losses. This paper summarizes and discusses experimental results on the effects of cathode-interconnect contacts on stack performance.