Total thermal neutron cross section measurements of hydrogen dense polymers from 0.0005–20 eV. (April 2023)

• Record Type: Journal Article
• Authors: Fritz, D.; Danon, Y.; Ramic, K.; Chapman, C.W.; Brown, J.M.; Arbanas, G.; Rapp, M.; Trumbull, T.H.; Zerkle, M.; Holmes, J.; Brain, P.; Ney, A.; Singh, S.; Cook, K.; Wang, B.
• Is Part Of: Annals of nuclear energy. Volume 183(2023)
• Publication Date: 2023-04
• Subjects: Polyethylene -- Polystyrene -- Plexiglas -- Total cross section -- Thermal scattering law; Nuclear energy -- Periodicals; Nuclear engineering -- Periodicals; 621.4805
• DOI: 10.1016/j.anucene.2022.109651
• Languages: English
• ISSNs: 0306-4549

Abstract

Abstract: Hydrogen dense polymers, specifically polyethylene, polystyrene, and Plexiglas, have served as neutron moderator and reflector materials in hundreds of separate critical benchmark experiments because of their low cost and abundance of hydrogen. In order to accurately model and simulate these critical benchmarks, the thermal scattering law (TSL) evaluation that governs how neutrons will thermalize must be well understood and rigorously validated. To support this validation, researchers at Rensselaer Polytechnic Institute performed total neutron cross section measurements for high-density polyethylene & polystyrene over the energy range 0.0005–20 eV and for Plexiglas G & Plexiglas G-UVT over the energy range 0.0005–3 eV. Comparisons were made between the measured cross section and that predicted by the ENDF/B-VIII.0 and Oak Ridge National Laboratory/European Spallation Source/Rensselaer Polytechnic Institute TSL evaluations for polyethylene, Plexiglas, and polystyrene, as available. These experiments represent the first total neutron cross section measurements for polystyrene.