Local inverse inelastic mean free path at interface. (1st November 2022)

• Record Type: Journal Article
• Authors: Pauly, Nicolas
• Is Part Of: Surface and interface analysis. Volume 55:Number 1(2023)
• Page Start: 52
• Page End: 62
• Publication Date: 2022-11-01
• Subjects: IMFP -- inelastic mean free path -- interface excitation -- local inverse inelastic mean free path; Surfaces (Physics) -- Periodicals; Surface chemistry -- Periodicals; Thin films -- Periodicals; 541.33
• DOI: 10.1002/sia.7159
• Languages: English
• ISSNs: 0142-2421

Abstract

Abstract : We calculated a local inverse inelastic mean free path (local‐IIMFP) for electrons crossing a medium–medium interface, considering various incident electron energies, crossing angles and combinations of materials. We used an extension of a classical dielectric model developed by Li and co‐workers for an electron crossing a surface (interface vacuum‐medium). Moreover, the integration over the distance of the local‐IIMFP allows to obtain the interface excitation parameter (or IEP) characterizing the change in excitation probability for an electron crossing an interface once caused by the presence of the interface in comparison with an electron for which only volume excitations are considered. We perform these calculations for angles between 0° and 80°, for electron energies between 500 and 2500 eV and for various pairs of materials, as Al/In for its academic interest or Au/Si and SiO2 /Si for their technological importance. Small but not negligible variations of the local‐IIMFP and the IEP were observed for metal–metal or metal–semiconductor interfaces, while quite significant variations are obtained when one of the materials is a insulator.