New Particle Formation and Growth to Climate‐Relevant Aerosols at a Background Remote Site in the Western Himalaya. Issue 7 (1st April 2021)

• Record Type: Journal Article
• Authors: Sebastian, Mathew; Kanawade, Vijay P.; Soni, Vijay K.; Asmi, Eija; Westervelt, Daniel. M.; Vakkari, Ville; Hyvärinen, Antti‐Pekka; Pierce, Jeffrey R.; Hooda, Rakesh K.
• Is Part Of: Journal of geophysical research. Volume 126:Issue 7(2021)
• Page Start: n/a
• Page End: n/a
• Publication Date: 2021-04-01
• Subjects: cloud condensation nuclei -- new particle formation -- particle growth -- the Himalaya; Atmospheric physics -- Periodicals; Geophysics -- Periodicals; 551.5
• DOI: 10.1029/2020JD033267
• Languages: English
• ISSNs: 2169-897X

Abstract

Abstract: New particle formation (NPF) can influence the Earth's radiative budget when the newly formed particles grow to climate‐relevant sizes. Here, we present analysis of 21 months of continuous aerosol size distribution measurements at a background remote site in the western Himalaya and provide observational evidence that newly formed particles grow to cloud condensation nuclei (CCN)‐active sizes (i.e., >20–100 nm in diameter). Out of total 55 NPF events, 38 (66%) events occurred in the pre‐monsoon season (March–May). NPF events were classified into those with and without pollution influence as polluted and cleaner, respectively, using black carbon data. The analysis of air mass age, based on the ratio of number concentration of Aitken to accumulation mode aerosols, indicated that NPF occurred in the relatively cleaner air masses reaching to the site. The median formation rate of 10 nm particles and particle growth rates for cleaner events were three‐fold and two‐fold, respectively, higher than polluted events. We present the first estimates of the survival probability of newly formed particles to 50 and 100 nm size, which was not attempted in an Indian environment previously. The survival probability to 50 nm particles ranged from 44% to 98%, with a mean and standard deviation of 82 ± 18%. On average, ∼60% of the particles surviving to 50 nm survived to 100 nm, making the overall survival probability of 100 nm to 53 ± 31%. This indicates that the probability of nucleated particles growing to CCN‐active sizes under a large source of condensing vapor (transported from nearby lower‐altitude regions) and low pre‐existing particle concentrations (background mountain site) is high compared to the previous studies. These findings highlight the importance of the efficiency of nucleation events for producing CCN, which is a critical basis of aerosol indirect effects. Key Points: We present new measurement‐based evidence of the contribution of new particle formation (NPF) to climate‐relevant aerosols in the Western Himalaya NPF occurred frequently in the pre‐monsoon (March–May) season NPF rates were higher for cleaner events than polluted events