Novel approach for low CO2 intensity hydrogen production from natural gas. Issue 21 (6th October 2022)

• Record Type: Journal Article
• Authors: Straus, Julian; Skjervold, Vidar Torarin; Anantharaman, Rahul; Berstad, David
• Is Part Of: Sustainable energy & fuels. Volume 6:Issue 21(2022)
• Page Start: 4948
• Page End: 4961
• Publication Date: 2022-10-06
• Subjects: Renewable energy sources -- Periodicals; Fuel cells -- Periodicals; Electric batteries -- Periodicals; Electrochemistry -- Periodicals; 660.297
• DOI: 10.1039/d2se00862a
• Languages: English
• ISSNs: 2398-4902

Abstract

Abstract : A reforming process for increased energy efficiency and CO2 capture rate through material recycling and CO2 liquefaction as separation technology. Abstract : Hydrogen from natural gas with CO2 capture can be a key transition technology to a low carbon energy system due to the abundance of natural gas and the possibility to increase the hydrogen production capacity quickly. However, it is necessary to achieve both a high energy efficiency and a high CO2 capture ratio for it to be a viable option. The liquefaction of CO2 is one promising separation technology as it provides the captured CO2 in a transportable format. This paper proposes a hydrogen production process with integrated CO2 liquefaction. Efficiencies of up to 84.7% (based on the higher heating value) and CO2 capture ratios of up to 97.2% can be achieved. One advantage of the utilization of CO2 liquefaction as separation technology is furthermore the possibility to incorporate a partial recycle of the flue gas from the separation to the water–gas shift reaction without additional equipment, increasing both energy efficiency and carbon capture ratio.