Design and performance evaluation of flexible tubular microreactor for methanol steam reforming reaction. (15th October 2022)

• Record Type: Journal Article
• Authors: Zhou, Shupan; Zhong, Yuchen; Lin, Weiming; You, Huihui; Li, Xinying; Wu, Linjing; Zhou, Wei
• Is Part Of: International journal of hydrogen energy. Volume 47:Number 85(2022)
• Page Start: 36022
• Page End: 36031
• Publication Date: 2022-10-15
• Subjects: Flexible microreactor -- Methanol steam reforming -- Hydrogen production -- Porous copper fiber material; Hydrogen as fuel -- Periodicals; Hydrogène (Combustible) -- Périodiques; Hydrogen as fuel; Periodicals; 665.81
• DOI: 10.1016/j.ijhydene.2022.08.194
• Languages: English
• ISSNs: 0360-3199

Abstract

Abstract: To obtain the flexible microreactor for potential application in constrained space, a novel flexible tubular microreactor was designed by using a corrugated shell and a high porosity porous copper fiber rod (PCFR) as catalyst support. The effect of placement position, bending direction, and bending angle on reaction performance of flexible tubular microreactor was investigated. Then, the stability of flexible tubular microreactor was further evaluated. The experimental results showed that the placement position and bending direction had a significant influence on the reaction performance of flexible tubular microreactor. Methanol conversion of flexible tubular microreactor with the vertical placement was 6.67% higher than that with horizontal placement. Higher methanol conversion and H2 flow rate were obtained when the microreactor bent along the vertical direction. The reaction performance of flexible tubular microreactor was found to decrease as the bending angle increased, and the methanol conversion decreased by around 14.07% with a bend of 90°. When the flexible tubular microreactor was horizontal placed with a bend of 60° in the vertical direction, the reaction performance of microreactor was not changed little after 20 cyclic bending. After continuous bending for 10 h, the methanol conversion and H2 flow rate of flexible tubular microreactor were 70.58% and 0.88 mol/h, showing good reaction performance. Highlights: A novel flexible tubular microreactor was developed. A high porosity porous copper fiber rod as catalyst support was designed. Effect of factors on reaction performance of the microreactor was investigated. Microreactor exhibited better hydrogen production performance under different bending conditions.