A broad study of tantalum strength from ambient to extreme conditions. (1st June 2022)

• Record Type: Journal Article
• Authors: Prime, Michael B.; Arsenlis, Athanasios; Austin, Ryan A.; Barton, Nathan R.; Battaile, Corbett C.; Brown, Justin L.; Burakovsky, Leonid; Buttler, William T.; Chen, Shuh-Rong; Dattelbaum, Dana M.; Fensin, Saryu J.; Flicker, Dawn G.; Gray, George T.; Greeff, Carl; Jones, David R.; Lane, J. Matthew D; Lim, Hojun; Luscher, D.J.; Mattsson, Thomas R.; McNaney, James M.; Park, Hye-Sook; Powell, Philip D.; Prisbrey, Shon T.; Remington, Bruce A.; Rudd, Robert E.; Sjue, Sky K.; Swift, Damian C.
• Is Part Of: Acta materialia. Volume 231(2022)
• Publication Date: 2022-06-01
• Subjects: Tantalum -- Strength -- Instabilities -- High pressure -- High strain rate; Materials -- Periodicals; Materials science -- Periodicals; Materials -- Mechanical properties -- Periodicals; Metallurgy -- Periodicals; Chemistry, Inorganic -- Periodicals; 620.112
• DOI: 10.1016/j.actamat.2022.117875
• Languages: English
• ISSNs: 1359-6454

Abstract

Graphical abstract: Abstract: By combining experiments and modeling from three US national laboratories, we explore compressive strength in a well-characterized material, tantalum, across pressures from zero to over 350 GPa, strain-rates from 10 − 3 /s to 10 8 /s and temperatures from 148 K to 3800 K. Strength values from 40+ experiments are shown to vary by nearly two orders of magnitude, from 0.15 GPa to over 10 GPa. Cross-comparison of these results allows pressure and strain-rate dependencies to be isolated, and strength increases more significantly with pressure than with strain rate over the range studied. Simulations using Preston-Tonks-Wallace, Livermore Multi-Scale, and Kink-Pair strength models test modeling capabilities and provide further insight into strength mechanics. The widely-used assumption in those models of shear-modulus scaling underpredicts strength by a factor of about two at extreme pressures in pulsed-power planar ramp-release experiments, which largely isolate pressure effects. Richtmyer-Meshkov Instability experiments, which largely isolate strain rate effects at ∼ 10 7 /s, suggest that modeling assumptions about mechanisms at the highest rates need further study. Laser-driven Rayleigh-Taylor instability experiments, which simultaneously probe extreme pressures and strain rates, provide both model and cross-platform experimental validation. The large-scale collaborative nature of this study covers a wide span of experimental conditions and modeling approaches, allowing for extraordinary insight into dynamic strength.