Cavity-melt partitioning of refractory radionuclides and implications for detecting underground nuclear explosions. (August 2020)

• Record Type: Journal Article
• Authors: Carrigan, Charles R.; Sun, Yunwei; Pili, Eric; Neuville, Daniel R.; Antoun, Tarabay
• Is Part Of: Journal of environmental radioactivity. Volume 219(2020)
• Publication Date: 2020-08
• Subjects: Radioxenon -- Underground nuclear explosion -- Noble gas transport -- CTBT International Monitoring System -- Atmospheric background -- Xenon isotopic evolution; Radioactivity -- Periodicals; Radiation, Background -- Periodicals; Radioecology -- Periodicals; Radioactive pollution -- Periodicals; Environmental Pollutants -- Periodicals; Radioactive Pollutants -- Periodicals; Radioactivity -- Periodicals; Radioécologie -- Périodiques; Pollution radioactive -- Périodiques; Fond de rayonnement -- Périodiques; 539.752
• DOI: 10.1016/j.jenvrad.2020.106269
• Languages: English
• ISSNs: 0265-931X

Abstract

Abstract: Isotopic ratios of radioxenon captured in the atmosphere can be indicators of the occurrence of an underground nuclear explosion. However, civilian sources of xenon isotopes, such as medical isotope production facilities and nuclear reactors, can interfere with detection of signals associated with nuclear testing, according to a standard model of the evolution of radioxenon isotopic abundances in a nuclear explosion cavity. We find that this standard model is idealized by not including the effects of physical processes resulting in the partitioning of the radionuclide inventory between a gas phase and rock melt created by the detonation and by ignoring seepage or continuous leakage of gases from the cavity or zone of collapse. Application of more realistic assumptions about the state of the detonation cavity results in isotopic activity ratios that differ from the civilian background more than the idealized standard model suggests, while also reducing the quantity of radioxenon available for atmospheric release and subsequent detection. Our simulations indicate that the physical evolution of the detonation cavity during the post-detonation partitioning process strongly influences isotopic evolution in the gas phase. Collapse of the cavity potentially has the greatest effect on partitioning of the refractory fission products that are precursors to radioxenon. The model allows for the possibility that post-detonation seismicity can be used to predict isotopic evolution. Highlights: New model evaluates post-detonation xenon isotopic evolution in nuclear test cavity. Isotopic ratios differ from background more than previously predicted. Seismic detection of cavity collapse allows bounding evolution of isotopic ratios.