Biomimetic and Biologically Compliant Soft Architectures via 3D and 4D Assembly Methods: A Perspective. Issue 16 (1st March 2022)

• Record Type: Journal Article
• Authors: Taylor, Jay M.; Luan, Haiwen; Lewis, Jennifer A.; Rogers, John A.; Nuzzo, Ralph G.; Braun, Paul V.
• Is Part Of: Advanced materials. Volume 34:Issue 16(2022)
• Page Start: n/a
• Page End: n/a
• Publication Date: 2022-03-01
• Subjects: 3D printing -- 4D fabrication -- biocompliant design -- biomimetic design -- directed assembly; Materials -- Periodicals; Chemical vapor deposition -- Periodicals; 620.11
• DOI: 10.1002/adma.202108391
• Languages: English
• ISSNs: 0935-9648

Abstract

Abstract: Recent progress in soft material chemistry and enabling methods of 3D and 4D fabrication—emerging programmable material designs and associated assembly methods for the construction of complex functional structures—is highlighted. The underlying advances in this science allow the creation of soft material architectures with properties and shapes that programmably vary with time. The ability to control composition from the molecular to the macroscale is highlighted—most notably through examples that focus on biomimetic and biologically compliant soft materials. Such advances, when coupled with the ability to program material structure and properties across multiple scales via microfabrication, 3D printing, or other assembly techniques, give rise to responsive (4D) architectures. The challenges and prospects for progress in this emerging field in terms of its capacities for integrating chemistry, form, and function are described in the context of exemplary soft material systems demonstrating important but heretofore difficult‐to‐realize biomimetic and biologically compliant behaviors. Abstract : Recent progress in soft material chemistry as it relates to direct ink writing and directed assembly through compressive buckling is discussed in relation to advances in 4D fabrication. The discussion focuses on the chemistry of important classes of soft materials, such as gels and elastomers, specifically in ways that allow new possibilities for biomimetic and biologically compliant forms of design.