A high-performance short-wave infrared phototransistor based on a 2D tellurium/MoS2 van der Waals heterojunction. Issue 38 (1st September 2021)

• Record Type: Journal Article
• Authors: Yao, Jinrong; Chen, Fangfang; Li, Juanjuan; Du, Junli; Wu, Di; Tian, Yongtao; Zhang, Cheng; Yang, Jinke; Li, Xinjian; Lin, Pei
• Is Part Of: Journal of materials chemistry. Volume 9:Issue 38(2021)
• Page Start: 13123
• Page End: 13131
• Publication Date: 2021-09-01
• Subjects: Materials -- Periodicals; Chemistry, Analytic -- Periodicals; Optical materials -- Research -- Periodicals; Electronics -- Materials -- Research -- Periodicals; 543.0284
• DOI: 10.1039/d1tc02502c
• Languages: English
• ISSNs: 2050-7526

Abstract

Abstract : A gate-tunable Te/MoS2 vdW heterostructure is fabricated, exhibiting favourable photodetection properties with a response spectrum covering the whole SWIR band. Abstract : Emerging two-dimensional semiconductors, particularly black phosphorus, have attracted great interest for their potential use in room-temperature and low-cost infrared photodetectors. Nevertheless, widespread application with black phosphorus has been substantially delayed by its lack of scalability and low environmental stability. Herein we report the hydrothermal synthesis of air-stable 2D tellurium with tunable thickness ranging from tens of nanometers down to 2.6 nm as well as the fabrication of a Te/MoS2 van der Waals heterojunction for a high-performance short-wave infrared (SWIR) photodetector. The heterostructure exhibits well-behaved field-effect transistor properties with a high ON/OFF ratio of over 10 7 and a steep subthreshold swing of 150 mV dec −1 . Due to the narrow bandgap of Te, the photodetector's response spectrum covers the whole SWIR band with a peak responsivity of 28.4 A W −1, 4.0 A W −1, and 0.87 A W −1 under 980 nm, 1.55 μm, and 3.0 μm illumination, respectively. Accordingly, detectivity up to 2.7 × 10 10 and 3.4 × 10 9 Jones is obtained at 980 nm and 1.55 μm wavelengths, respectively. These findings demonstrate the potential of 2D Te as a new platform for realizing room-temperature SWIR photodetectors. Besides, our study can serve as a reference for other vdW structure designs, thus expanding the research scope for 2D Te-based optoelectronics.