Insights from application of a hierarchical spatio-temporal model to an intensive urban black carbon monitoring dataset. (15th May 2022)

• Record Type: Journal Article
• Authors: Wai, Travis Hee; Apte, Joshua S.; Harris, Maria H.; Kirchstetter, Thomas W.; Portier, Christopher J.; Preble, Chelsea V.; Roy, Ananya; Szpiro, Adam A.
• Is Part Of: Atmospheric environment. Volume 277(2022)
• Publication Date: 2022-05-15
• Subjects: Black Carbon -- Spatiotemporal Modeling -- Exposure Assessment -- Fine Scale Prediction; Air -- Pollution -- Periodicals; Air -- Pollution -- Meteorological aspects -- Periodicals; 551.51
• DOI: 10.1016/j.atmosenv.2022.119069
• Languages: English
• ISSNs: 1352-2310

Abstract

Abstract: Existing regulatory pollutant monitoring networks rely on a small number of centrally located measurement sites that are purposefully sited away from major emission sources. While informative of general air quality trends regionally, these networks often do not fully capture the local variability of air pollution exposure within a community. Recent technological advancements have reduced the cost of sensors, allowing air quality monitoring campaigns with high spatial resolution. The 100 × 100 black carbon (BC) monitoring network deployed 100 low-cost BC sensors across the 15 km 2 West Oakland, CA community for 100 days in the summer of 2017, producing a nearly continuous site-specific time series of BC concentrations which we aggregated to 1-h averages. Leveraging this dataset, we employed a hierarchical spatio-temporal model to accurately predict local spatio-temporal concentration patterns throughout West Oakland, at locations without monitors (average cross-validated hourly temporal R 2 = 0.60). Using our model, we identified spatially varying temporal pollution patterns associated with small-scale geographic features and proximity to local sources. In a sub-sampling analysis, we demonstrated that fine scale predictions of nearly comparable accuracy can be obtained with our modeling approach by using ∼30% of the 100 × 100 BC network supplemented by a shorter-term high-density campaign. Highlights: Hourly black carbon concentration maps predicted in West Oakland in summer 2017. Leveraged data from the intensive 100 × 100 monitoring campaign. Advanced spatiotemporal model can produce similar results with less intensive data. Sources and geographic features predict spatial variation in diurnal pollution.