Accurate real-time monitoring of fine dust using a densely connected convolutional networks with measured plasma emissions. (April 2022)

• Record Type: Journal Article
• Authors: Yang, Jun-Ho; Park, Sanghoon; Kim, Seonghwan; Cho, Youngkyu; Yoh, Jack J.
• Is Part Of: Chemosphere. Volume 293(2022)
• Publication Date: 2022-04
• Subjects: Deep learning -- DenseNet -- Spark-induced plasma spectroscopy -- Fine dust -- Source identification; Pollution -- Periodicals; Pollution -- Physiological effect -- Periodicals; Environmental sciences -- Periodicals; Atmospheric chemistry -- Periodicals; 551.511
• DOI: 10.1016/j.chemosphere.2022.133604
• Languages: English
• ISSNs: 0045-6535

Abstract

Abstract: Accurate identification and monitoring of fine dust are emerging as a primary global issue for addressing the harmful effects of fine dust on public health. Identifying the source of fine dust is indispensable for ensuring the human lifespan as well as preventing environmental disasters. Here a simple yet effective spark-induced plasma spectroscopy (SIPS) unit combined with deep learning for real-time classification is verified as a fast and precise PM (particulate matter) source identification technique. SIPS promises portable use, label-free detection, source identification, and chemical susceptibility in a single step with acceptable speed and accuracy. In particular, the densely connected convolutional networks (DenseNet) are used with measured spark-induced plasma emission datasets to identify PM sources at above 98%. The identification performance was compared with other common classification methods, and DenseNet with dropouts (30%), optimized batch size (16), and cyclic learning rate training emerged as the most promising source identification method. Graphical abstract: Image 1 Highlights: Accurate (>98%) identification of fine dust is achieved by using SIPS. Application of deep learning in SIPS is conducted for the first time. SIPS combined with DenseNet offered the best identification for fine dust sources.