An analysis of high fine aerosol loading episodes in north-central Spain in the summer 2013 - Impact of Canadian biomass burning episode and local emissions. (July 2018)

• Record Type: Journal Article
• Authors: Burgos, M.A.; Mateos, D.; Cachorro, V.E.; Toledano, C.; de Frutos, A.M.; Calle, A.; Herguedas, A.; Marcos, J.L.
• Is Part Of: Atmospheric environment. Volume 184(2018)
• Page Start: 191
• Page End: 202
• Publication Date: 2018-07
• Subjects: Fine aerosol particles -- Biomass burning -- Anthropogenic pollution -- Aerosol microphysical properties -- Aerosol optical properties -- Aerosol radiative effect; Air -- Pollution -- Periodicals; Air -- Pollution -- Meteorological aspects -- Periodicals; 551.51
• DOI: 10.1016/j.atmosenv.2018.04.024
• Languages: English
• ISSNs: 1352-2310

Abstract

Abstract: This work presents an evaluation of a surprising and unusual high turbidity summer period in 2013 recorded in the north-central Iberian Peninsula (IP). The study is made up of three main pollution episodes characterized by very high aerosol optical depth (AOD) values with the presence of fine aerosol particles: the strongest long-range transport Canadian Biomass Burning (BB) event recorded, one of the longest-lasting European Anthropogenic (A) episodes and an extremely strong regional BB. The Canadian BB episode was unusually strong with maximum values of AOD(440 nm) ∼ 0.8, giving rise to the highest value recorded by photometer data in the IP with a clearly established Canadian origin. The anthropogenic pollution episode originated in Europe is mainly a consequence of the strong impact of Canadian BB events over north-central Europe. As regards the local episode, a forest fire in the nature reserve near the Duero River (north-central IP) impacted on the population over 200 km away from its source. These three episodes exhibited fingerprints in different aerosol columnar properties retrieved by sun-photometers of the AErosol RObotic NETwork (AERONET) as well as in particle mass surface concentrations, PMx, measured by the European Monitoring and Evaluation Programme (EMEP). Main statistics, time series and scatterplots relate aerosol loads (aerosol optical depth, AOD and particulate matter, PM) with aerosol size quantities (Ångström Exponent and PM ratio). More detailed microphysical/optical properties retrieved by AERONET inversion products are analysed in depth to describe these events: contribution of fine and coarse particles to AOD and its ratio (the fine mode fraction), volume particle size distribution, fine volume fraction, effective radius, sphericity fraction, single scattering albedo and absorption optical depth. Due to its relevance in climate studies, the aerosol radiative effect has been quantified for the top and bottom of the atmosphere, obtaining mean daily values for this extraordinary summer period of −14.5 and −47.5 Wm −2, respectively. Highlights: Evaluation of the summer period with highest fine aerosol occurrence and intensity. Aerosol load and size used to establish the length and intensity of each episode. Fine pollution unexpectedly represents 75% of the summer intrusions. Aerosol radiative effect: −14.5/−47.5 Wm −2 at the top/bottom of the atmosphere.