Inducing thermionic emission from lanthanum hexaboride probes in Magnum-PSI. (December 2021)

• Record Type: Journal Article
• Authors: van den Berg-Stolp, J.; Classen, I.G.J.; van der Meiden, H.J.; Vernimmen, J.W.M.; Brons, S.; van Rooij, G.J.
• Is Part Of: Nuclear materials and energy. Volume 29(2021)
• Publication Date: 2021-12
• Subjects: Thermionic emission -- Inverse sheath regime -- Lanthanum hexaboride -- Linear plasmas -- Self-sputtering; Nuclear energy -- Periodicals; Nuclear fuels -- Periodicals; Nuclear reactors -- Materials -- Periodicals; Radioactive substances -- Periodicals; 621.4833
• DOI: 10.1016/j.nme.2021.101097
• Languages: English
• ISSNs: 2352-1791

Abstract

Abstract: For thermionic emission rates exceeding the incident plasma electron flux, recent theory proposes an inverse sheath regime, with promising properties for future application in fusion edge plasmas. With the aim of inducing thermionic emission in fusion-relevant plasma conditions, several lanthanum hexaboride probes were heated in the linear plasma generator Magnum-PSI. During exposures at low plasma power and additional pulsed laser heating, the probe's floating potential was reduced by up to 12%, providing a possible indication of thermionic emission. However, these observations coincided with rapid erosion of probe material, attributed to enhanced lanthanum self-sputtering. During follow-up experiments with helium plasmas at electron temperatures around 1 eV, the lanthanum ion impact energy and sputtering yield were reduced, and rapid erosion was avoided, thus confirming the thesis of self-sputtering. A parameter scan of plasma power resulted in LaB 6 surface temperatures up to 2450 °C, exceeding the theoretical inverse sheath threshold temperature by over 300 °C. However, the probe's floating potential did not deviate from reference measurements using a probe with high electronic work function, indicating absence of strong thermionic emission. This apparent discrepancy is attributed to the effects of probe surface modifications as observed during these experiments: impurity deposition, erosion and cavity formation. These modifications possibly affected the LaB 6 electronic work function, thereby keeping the inverse sheath threshold out of reach. In conclusion, although LaB 6 has one of the lowest work functions available, the inverse sheath threshold conditions could not be reached with the present setup in Magnum-PSI. Surface modifications thus do form a limiting factor for the application of LaB 6 in fusion-relevant plasma conditions. Moreover, the window of stable operation for LaB 6 in dense hydrogen plasmas is limited below ∼ 1.5 eV, and does not overlap with the conditions expected in the edge region of future fusion devices like ITER. Highlights: LaB 6 probes were heated up to 2450 °C under fusion-relevant plasma conditions. Surface modifications limit the effective operation of powder-pressed LaB 6 . Lanthanum self-sputtering in dense plasma conditions leads to rapid erosion. The LaB 6 operation window does not overlap with ITER divertor conditions.