Provenancing of cement using elemental analyses and isotope techniques – the state-of-the-art and future perspectives. Issue 10 (10th September 2021)

• Record Type: Journal Article
• Authors: Kazlagić, Anera; Vogl, Jochen; Gluth, Gregor J. G.; Stephan, Dietmar
• Is Part Of: Journal of analytical atomic spectrometry. Volume 36:Issue 10(2021)
• Page Start: 2030
• Page End: 2042
• Publication Date: 2021-09-10
• Subjects: Atomic spectra -- Periodicals; Atomic absorption spectroscopy -- Periodicals; 543.0858
• DOI: 10.1039/d1ja00144b
• Languages: English
• ISSNs: 0267-9477

Abstract

Abstract : The use of elemental analyses and isotope techniques for cement provenancing are reviewed. Based on the currently available data and approaches from related fields, future perspectives and a combined approach for cement provenancing are outlined. Abstract : With the aim of identifying the origin and the manufacturer of a cement, a reliable procedure that provides unambiguous results is needed. Such procedure could resolve practical issues in damage research, liability issues and forensic investigations. A substantial number of attempts for fingerprinting of building materials, including cement, has already been carried out during the last decades. Most of them were based on concentration analysis of the main elements/components. This review provides an overview of provenance studies of cement and the main approaches commonly used. Provenance studies of cement via isotope techniques are also presented and discussed as representatives of the state-of-the-art in the field. Due to the characteristic properties and the occurrence of carefully selected isotope ratios, unique fingerprints of different kinds of materials can be provided by these methods. This property has largely been explored in various scientific fields such as geo- and cosmochemistry, food forensics, archaeology, geochronology, biomedical studies, and climate change processes. However, the potential of isotope techniques in cement and concrete research for provenance studies has barely been investigated. Therefore, the review outlines a suitable approach using isotope ratios, which could lead to reliable provenancing of cementitious materials in the future.