Solar chimney power plant integrated with a photocatalytic reactor to remove atmospheric methane: A numerical analysis. (15th September 2021)

• Record Type: Journal Article
• Authors: Ming, Tingzhen; Gui, Haoyu; Shi, Tianhao; Xiong, Hanbing; Wu, Yongjia; Shao, Yimin; Li, Wei; Lu, Xiaohua; de Richter, Renaud
• Is Part Of: Solar energy. Volume 226(2021)
• Page Start: 101
• Page End: 111
• Publication Date: 2021-09-15
• Subjects: Non-CO2 greenhouse gas removal -- Photocatalytic reactor -- Solar chimney power plant -- Numerical simulation -- Global warming; Solar energy -- Periodicals; Solar engines -- Periodicals; 621.47
• DOI: 10.1016/j.solener.2021.08.024
• Languages: English
• ISSNs: 0038-092X

Abstract

Highlights: The numerical simulation is used to validate the effectiveness of atmospheric methane removal by SCPP-PCR. The performance and influencing factors of photocatalytic oxidation of methane by the SCPP-PCR were analyzed. The photocatalytic efficiency and purification rate were introduced to evaluate the effect of SCPP-PCR on methane removal. The optimum dimension of photocatalytic reactor with pore diameters of 2–4 mm was determined. Abstract: Methane (CH4 ) is the second largest contributor to global warming among all greenhouses gases. A solar chimney power plant integrated with a photocatalytic reactor (SCPP-PCR) is a promising large-scale method for removing CH4 from the atmosphere. This study used computational fluid dynamics (CFD) to investigate the performance and factors influencing photocatalytic oxidation of methane by the SCPP-PCR system. The geometry of a SCPP is the same as the prototype of the SCPP built in Manzanares (Spain). The PCR is designed based on a honeycomb monolith photoreactor. The numerical results revealed that the SCPP-PCR system can degraded 21, 312 g methane per day with the actual solar radiation data when the channel diameter of the honeycomb PCR was 4 mm and channel length was 8 m. Although increasing the length or decreasing the channel diameter of the PCR would improve photocatalytic efficiency, the rate of airflow of the system would be reduced. The maximum methane purification rate of the SCPP-PCR system was determined.