Syngas production by methane-rich combustion in a divergent burner of porous media. (1st July 2021)

• Record Type: Journal Article
• Authors: Dai, Huaming; Zhu, Huiwei; Dai, Hongchao; Song, Ziwei; Wang, Zhiqiang; He, Song; Wang, Xinyi
• Is Part Of: International journal of hydrogen energy. Volume 46:Number 45(2021)
• Page Start: 23279
• Page End: 23291
• Publication Date: 2021-07-01
• Subjects: Coal mine methane -- Divergent porous media -- Methane reforming -- Flame stability limit -- Energy conversion efficiency; Hydrogen as fuel -- Periodicals; Hydrogène (Combustible) -- Périodiques; Hydrogen as fuel; Periodicals; 665.81
• DOI: 10.1016/j.ijhydene.2021.04.160
• Languages: English
• ISSNs: 0360-3199

Abstract

Abstract: The superadiabatic combustion in porous media contributes to the efficient conversion of methane to syngas. In this paper, a divergent packed bed burner of two-layer was proposed to obtain the characteristics of methane partial oxidation. The divergent angle, interface location and pellet diameter were used to study the temperature and species distributions. Results indicate that the upper limit of velocity gradually decreased as the equivalence ratio increased and the limit of the divergent burner is obviously higher than that of the cylindrical one. The increasing of the divergent angle within a certain range enhances the methane conversion and the 15° shows the best among the selected five angles. The mole fractions of H2 and CO gradually decrease when the interface locations move from the cylindrical region to the divergent one. As the equivalence ratio increased from 1.3 to 3.5, the yields of H2 and CO and the energy conversion efficiency of syngas increase first and then decrease, and the maximum efficiency of 45.9% appears at the equivalence ratio of 2.0. The divergent region weakens the influence of inlet velocities and contributes to the stability of reforming reactions. Graphical abstract: Image 1 Highlights: A divergent packed bed burner of two layers was designed. Upper limit of velocity decreased with the increasing of equivalence ratio. H2 and CO fractions decrease as interface location moves to divergent one. Divergent structure contributes to the reforming stability.