Experimental study of concrete activation compared to MCNP simulations for safety of neutron sources. (May 2021)

• Record Type: Journal Article
• Authors: Hajdú, D.; Dian, E.; Gméling, K.; Klinkby, E.; Cooper-Jensen, C.P.; Osán, J.; Zagyvai, P.
• Is Part Of: Applied radiation and isotopes. Volume 171(2021)
• Publication Date: 2021-05
• Subjects: ESS -- Neutron activation -- Concrete activation -- MCNP -- Neutron shielding -- Cinder; Radiology -- Periodicals; Radiation -- Industrial applications -- Periodicals; Nuclear chemistry -- Periodicals; Internet resource; Periodical; 660.298
• DOI: 10.1016/j.apradiso.2021.109644
• Languages: English
• ISSNs: 0969-8043

Abstract

Abstract: The neutron activation of shielding materials and the generated decay gamma radiation are well-known issues in terms of occupational exposure. Though the trace elements of shielding concretes can be dominant sources of the produced activity in such cases, their concentrations are often missing from the input data of shielding-related Monte Carlo simulations. For this reason, three concrete types were studied, that were considered in the European Spallation Source (ESS) ERIC. Their composition – including the trace elements – were determined via XRF, PGAA and NAA techniques. Realistic input data were developed for these materials, containing the parent elements of all the dominant radioisotopes, and were validated against measured data of neutron irradiation experiments. Highlights: The most important gamma-emitting isotopes from neutron activation were determined in concrete samples. Measurement-based material compositions were assembled for MCNP simulations. MCNP and Cinder activation simulation results were validated against measurements. Activation related safety considerations were presented via a European Spallation Source operational scenario.