Overcoming challenges to support us resumption of high specific activity cobalt-60. (March 2021)

• Record Type: Journal Article
• Authors: Howard, R.H.; Reichenberger, M.A.; Urban-Klaehn, J.M.; Peterson-Droogh, J.L.; Brookman, J.V.; Gross, B.; Tyler, C.; Navarro, J.; Lillo, M.; Zillmer, A.
• Is Part Of: Applied radiation and isotopes. Volume 169(2021)
• Publication Date: 2021-03
• Subjects: HSA Co-60 -- Reactor produced radioisotopes -- Target design -- Advanced test reactor; Radiology -- Periodicals; Radiation -- Industrial applications -- Periodicals; Nuclear chemistry -- Periodicals; Internet resource; Periodical; 660.298
• DOI: 10.1016/j.apradiso.2020.109494
• Languages: English
• ISSNs: 0969-8043

Abstract

Abstract: Domestic production of high specific activity 60 Co was halted after a target rupture in 2012 at the Advanced Test Reactor (ATR). The Isotope Program (IP) within the US Department of Energy (DOE) Office of Science tasked a multilaboratory team of researchers and managers from Oak Ridge and Idaho National Laboratories with the redesign the radioisotope capsule. The objective of this effort was to create a more robust and reliable design, compared to the pre-2012 target. The team successfully completed this task to produce the DOE-IP cobalt (Co) production capsule design. Furthermore, 66 capsules were successfully fabricated by Oak Ridge National Laboratory (ORNL) and delivered to Idaho National Laboratory (INL) for irradiation in the ATR between January 2014 and October 2016. This paper describes the efforts of the team to prepare and disposition the two initial DOE-IP Co production capsules that were processed in March 2020. These efforts include performing accurate production predictions, experimentally validating predictions with assay measurements, shipping with the Orano-furnished Battelle Energy Alliance Research Reactor shipping package, and disassembling capsules at the isotope vendor site. Highlights: The work details the work to redesign and disposition a new high specific activity Co-60 production capsule. The experiment contains 42g of feedstock and is designed to reach up 300 Ci/g Co-60. The manuscript describes a sound process to analyze, assay, and process capsules to support the U.S. production of HSA Co-60.