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Coherent control for separation of the librational response through the ultrafast optically-heterodyne-detected optical- Kerr-effect (OHD-OKE). (May 2016)
Record Type:
Journal Article
Title:
Coherent control for separation of the librational response through the ultrafast optically-heterodyne-detected optical- Kerr-effect (OHD-OKE). (May 2016)
Main Title:
Coherent control for separation of the librational response through the ultrafast optically-heterodyne-detected optical- Kerr-effect (OHD-OKE)
Abstract: We report the first experiment results on selective spectroscopy of librational response in ortho-dichlorobenzene at room temperature. By optimization of the controlling parameters we have achieved the suppression of the Raman-active vibrational and orientational responses. We have used the two-pulse excitation scheme. The controlling parameters were pulse duration, intensity and delay between two pump pulses.