A stabilized PEO-based solid electrolyte via a facile interfacial engineering method for a high voltage solid-state lithium metal battery. Issue 42 (17th April 2020)

• Record Type: Journal Article
• Authors: Qiu, Jiliang; Yang, Lufeng; Sun, Guochen; Yu, Xiqian; Li, Hong; Chen, Liquan
• Is Part Of: Chemical communications. Volume 56:Issue 42(2020)
• Page Start: 5633
• Page End: 5636
• Publication Date: 2020-04-17
• Subjects: Chemistry -- Periodicals; 540
• DOI: 10.1039/d0cc01829e
• Languages: English
• ISSNs: 1359-7345

Abstract

Abstract : A facile interfacial engineering method was developed to achieve stable cycling of a Li/PEO–LiTFSI/LiNi0.5 Co0.2 Mn0.3 O2 solid-state battery at 4.2 V. Abstract : A facile interfacial engineering method via in situ electro-deposition was developed to stabilize the PEO-based solid electrolyte in high voltage solid-state lithium metal batteries (Li/PEO–LiTFSI/LiNi0.5 Co0.2 Mn0.3 O2 ), which demonstrate a superior capacity retention of 72.3% after 200 cycles in 3.0–4.2 V. The critical factors for the interfacial engineering method were also demonstrated in this study.