Abstract : In article number 2001859, Wei Wang, Zongping Shao, and co‐workers present in situ exsolved NiCo alloy nanoparticles exhibiting high specific surface areas and strong interaction with the La0.55 Sr0.30 TiO3−δ perovskite substrate, thus leading to the superior electrochemical activity for NH3 decomposition and excellent antisintering capability of the composite anode. Cover illustrator: Yijun Zhong.