Effect of differential diffusion on turbulent lean premixed hydrogen enriched flames through structure analysis. (1st April 2020)

• Record Type: Journal Article
• Authors: Zhang, Weijie; Wang, Jinhua; Lin, Wenjun; Mao, Runze; Xia, Hao; Zhang, Meng; Huang, Zuohua
• Is Part Of: International journal of hydrogen energy. Volume 45:Number 18(2020)
• Page Start: 10920
• Page End: 10931
• Publication Date: 2020-04-01
• Subjects: Lean premixed flames -- Hydrogen combustion -- Differential diffusion -- Flame structure -- Turbulent burning velocity; Hydrogen as fuel -- Periodicals; Hydrogène (Combustible) -- Périodiques; Hydrogen as fuel; Periodicals; 665.81
• DOI: 10.1016/j.ijhydene.2020.02.032
• Languages: English
• ISSNs: 0360-3199

Abstract

Abstract: This study presents the flame structure influenced by the differential diffusion effects and evaluates the structural modifications induced by the turbulence, thus to understand the coupling effects of the diffusively unstable flame fronts and the turbulence distortion. Lean premixed CH4 /H2 /air flames were conducted using a piloted Bunsen burner. Three hydrogen fractions of 0, 30% and 60% were adopted and the laminar flame speed was kept constant. The turbulence was generated with a single-layer perforated plate, which was combined with different bulk velocities to obtain varied turbulence intensities. Quasi-laminar flames without the plate were also performed. Explicit flame morphology was obtained using the OH-PLIF. The curvature, flame surface density and turbulent burning velocity were measured. Results show that the preferential transport of hydrogen produces negatively curved cusps flanked with positively curved bulges, which are featured by skewed curvature pdfs and consistent with the typical structure caused by the Darrieus-Landau instability. Prevalent bulge-cusp like wrinkles remain with relatively weak turbulence. However, stronger turbulence can break the bulges to be finer, and induce random positively curved cusps, therefore to destroy the bulge-cusp structures. Evident positive curvatures are generated in this process modifying the skewed curvature pdfs to be more symmetric, while the negative curvatures are not affected seriously. From low to high turbulence intensities, the hydrogen addition always strengthens the flame wrinkling. The augmentation of flame surface density and turbulent burning velocity with hydrogen is even more obvious at higher turbulence intensity. It is suggested that the differential diffusion can persist and even be strengthened with strong turbulence. Highlights: Coupling effects of the dfferential diffusion and turbulence were conducted. Preferential H2 transport produces bulge-cusp structures similar to the DL instability. Turbulence enhances the wrinkling mainly by influencing the positively curved flamelet. Dfferential diffusion effects are even strengthened at higher turbulence intensity.