Toward anthropogenic combustion emission constraints from space‐based analysis of urban CO2/CO sensitivity. Issue 18 (23rd September 2013)

• Record Type: Journal Article
• Authors: Silva, Sam J.; Arellano, Avelino F.; Worden, Helen M.
• Is Part Of: Geophysical research letters. Volume 40:Issue 18(2013:Sep.)
• Page Start: 4971
• Page End: 4976
• Publication Date: 2013-09-23
• Subjects: megacities -- anthropogenic combustion -- emissions -- enhancement ratios -- MOPITT CO -- GOSAT/ACOS CO2; Geophysics -- Periodicals; Planets -- Periodicals; Lunar geology -- Periodicals; 550
• DOI: 10.1002/grl.50954
• Languages: English
• ISSNs: 0094-8276

Abstract

Abstract : [1] We explore the value of multispectral CO retrievals from NASA/Terra Measurement of Pollution In The Troposphere (MOPITT v5), along with Atmospheric CO2 Observations from Space (ACOSv2.9) CO2 retrievals from the Japan Aerospace Exploration Agency Greenhouse Gases Observing Satellite (GOSAT), for characterizing emissions from anthropogenic combustion. We use these satellite retrievals to analyze observed CO2 /CO enhancement ratios (ΔCO2 /ΔCO) over megacities. Since CO is coemitted with CO2 in anthropogenic combustion, the observed ΔCO2 /ΔCO characterizes the general trend in combustion activity. Our analyses show patterns in ΔCO2 /ΔCO that correspond well with the developed/developing status of megacities, and ΔCO2 /ΔCO that agree well with available literature and emission inventories to approximately 20%. Comparisons with ΔCO2 /ΔCO derived from Total Carbon Column Observing Network measurements show similar agreement, where some of the differences in observed ΔCO2 /ΔCO are due to representativeness and limited GOSAT data. Our results imply potential constraints in anthropogenic combustion from GOSAT/MOPITT, particularly in augmenting our carbon monitoring systems. Key Points: Space‐based CO2/CO ratios offer constraints on anthropogenic combustion Combustion‐related retrievals can augment carbon monitoring systems Satellite‐derived combustion patterns are consistent to literature and other data