A quantum mechanical exploration of phonon energy-loss spectroscopy using electrons in the aloof beam geometry. (13th November 2017)

• Record Type: Journal Article
• Authors: Allen, L J; Brown, H G; Findlay, S D; Forbes, B D
• Is Part Of: Microscopy. Volume 67(2018)Supplement 1
• Page Start: i24
• Page End: i29
• Publication Date: 2017-11-13
• Subjects: electron energy-loss spectroscopy -- phonon excitation -- aloof beam geometry; Microscopy -- Periodicals; 502.825
• DOI: 10.1093/jmicro/dfx038
• Languages: English
• ISSNs: 2050-5698

Abstract

Abstract : Phonon energy-loss spectroscopy using electrons has both short-range (high resolution) and long-range (low resolution) components. We discuss how these two contributions arise from a fundamental quantum mechanical perspective. The long-range interaction dominates in aloof beam imaging, a mode in which radiation damage can be avoided. Abstract: Phonon energy-loss spectroscopy using electrons has both high resolution and low resolution components, associated with short- and long-range interactions, respectively. In this paper, we discuss how these two contributions arise from a fundamental quantum mechanical perspective. Starting from a correlated model for the atomic motion we show how short range 'impact' scattering and long range 'dipole' scattering arises. The latter dominates in aloof beam imaging, an imaging geometry in which radiation damage can be avoided.