Assessment on temperature-pressure severally controlled explosion pretreatment of poplar. (15th February 2020)

• Record Type: Journal Article
• Authors: Wang, Huimei; Liu, Zhong; Zheng, Xu; Pan, Xuejun; Hui, Lanfeng; Li, Jingzhi; Zhang, Hao
• Is Part Of: Carbohydrate polymers. Volume 230(2020)
• Publication Date: 2020-02-15
• Subjects: Cellulose -- Hemicellulose -- Lignin -- Temperature-pressure severally controlled explosion -- Enzymatic -- Hydrolysis; Polysaccharides -- Periodicals; Polysaccharides -- Periodicals; Polysaccharides -- Périodiques; Electronic journals; 547.78
• DOI: 10.1016/j.carbpol.2019.115622
• Languages: English
• ISSNs: 0144-8617

Abstract

Graphical abstract: Highlights: Temperature-pressure severally controlled explosion was proposed to pretreat poplar. Temperature was controlled by partial steam pressure, with pressure adjusted by N2 . When pressure increased, there was an improvement of cellulose conversion yield. Micro-CT was used to explore the changes of cross-section and 3D structure. Abstract: In this work, temperature-pressure severally controlled explosion pretreatment (TPE) was proposed to pretreat poplar chips to improve the cellulase hydrolysis yield. In TPE process, native poplar chips (NP) were mixed with steam and N2 under pressure of 2.6, 2.8 and 3.0 MPa at 209 °C for 7 min. Meanwhile, steam explosion (SE) was also used to pretreat poplar chips for comparison at 209 °C (1.9 MPa) for 7 min. Results showed that the contents of hemicellulose and lignin were decreased from 19.4 % to 4.6 % and from 27.8 %–19.5 % with increasing pressure, respectively. For cellulase hydrolysis process, TPE was more advantageous than SE due to lower contents of hemicellulose and lignin, resulting in a higher cellulose conversion (40.7 %) in relation to SE sample (34.9 %). The Langmuir isothermal- type equation expressed the factors related to the hydrolysis capacity, and the results showed that this model can well describe the kinetics of the enzymatic hydrolysis.