99Mo recoil atoms yield in the 100Mo(p, x) reaction on cyclotron irradiation of Mo nanofilms. (2nd July 2019)

• Record Type: Journal Article
• Authors: Artyukhov, Aleksei Aleksandrovich; Zagriadsky, Vladimir Anatolevich; Kravets, Iakov Maksimovich; Kuznetsova, Tatiana Mikhailovna; Latushkin, Sergei Terentevich; Menshikov, Leonid Ieronimovich; Udalova, Tatiana Andreevna; Chuvilin, Dmitrii Iurevich
• Other Names: Elbert Tomas guestEditor.; Lawrie Kenneth guestEditor.
• Is Part Of: Journal of labelled compounds & radiopharmaceuticals. Volume 62:Number 11(2019)
• Page Start: 803
• Page End: 808
• Publication Date: 2019-07-02
• Subjects: isotope separation -- molybdenum‐99 -- nanolayers -- Szilard‐Chalmers effect -- yield of recoil atoms; Tracers (Chemistry) -- Periodicals; Radiopharmaceuticals -- Periodicals; 615.8424
• DOI: 10.1002/jlcr.3737
• Languages: English
• ISSNs: 0362-4803

Abstract

Abstract : We study the possibility of increasing the specific activity of 99 Mo produced by irradiating molybdenum targets with the use of the Szilard‐Chalmers effect. According to the Szilard‐Chalmers effect, recoil atoms of the 99 Mo radionuclide can be produced in nuclear reactions and retained in surrounding buffer substance. The objective of our work is to measure the yield of recoil atoms in the buffer as a function of the molybdenum layer thickness. The yield of recoil 99 Mo atoms in the 100 Mo(p, x) 99 Mo nuclear reaction as a function of metallic molybdenum nanolayer thickness has been measured. Measurements were carried out after irradiation of nanolayers in the U‐150 cyclotron with 28‐MeV protons. Nanolayers of molybdenum with thickness of 30 to 220 nm were produced by magnetron sputtering on sapphire plates. The yield of the mass of 99 Mo recoil atoms was found to be the highest with the molybdenum layer thickness of 80 ± 5 nm. The enrichment factor (EF) has been defined as a ratio of the 99 Mo collector specific activity (SA) to the entire target SA before separation as EF = 1200 ± 150. The specific activity of 99 Mo produced in the collector was estimated to be approximately equal to 25 Ci·g −1 . Abstract : We have found that the yield of the mass of 99 Mo recoil atoms produced by irradiating molybdenum targets with 28 MeV protons is the highest with the molybdenum layer thickness of 80 ± 5 nm. The enrichment factor (EF) has been defined as a ratio of the 99 Mo collector specific activity (SA) to the entire target SA before separation as EF = 1200 ± 150.