Time-dependent shear rate inhomogeneities and shear bands in a thixotropic yield-stress fluid under transient shear. Issue 39 (23rd September 2019)

• Record Type: Journal Article
• Authors: Wei, Yufei; Solomon, Michael J.; Larson, Ronald G.
• Is Part Of: Soft matter. Volume 15:Issue 39(2019)
• Page Start: 7956
• Page End: 7967
• Publication Date: 2019-09-23
• Subjects: Soft condensed matter -- Periodicals; 530.413
• DOI: 10.1039/c9sm00902g
• Languages: English
• ISSNs: 1744-683X

Abstract

Abstract : We study the rheological responses and shear-rate inhomogeneities and shear banding behaviors of a thixotropic fumed silica suspension in shear startup tests and flow reversal tests. Abstract : We study the rheological responses and shear-rate inhomogeneities and shear banding behaviors of a thixotropic fumed silica suspension in shear startup tests and flow reversal tests. We find that this suspension under transient shear exhibits not only viscoelasticity, yielding, kinematic hardening, and thixotropy, but also time-dependent shear inhomogeneities including bands when the apparent shear rate is below a critical value between 0.1 and 0.25 s −1 . Through multiple shear startup tests and flow reversal tests, we find that thixotropy promotes flow heterogeneity while kinematic hardening suppresses it. We propose a simple thixo-plastic constitutive equation that can qualitatively predict the important features of the rheological response and banding dynamics in shear startup tests and flow reversal tests.