Modeling and Design of a Catalytic Wall Reactor for the Methanation of Carbon Dioxide. Issue 5 (25th March 2018)

• Record Type: Journal Article
• Authors: Gruber, Manuel; Wieland, Christoph; Habisreuther, Peter; Trimis, Dimosthenis; Schollenberger, Dominik; Bajohr, Siegfried; vonMorstein, Olaf; Schirrmeister, Steffen
• Other Names: Klemm Elias guestEditor.; Sauer Jörg guestEditor.
• Is Part Of: Chemie Ingenieur Technik. Volume 90:Issue 5(2018)
• Page Start: 615
• Page End: 624
• Publication Date: 2018-03-25
• Subjects: CO2 methanation -- Microprocess engineering -- Power‐to‐gas -- Reactor modeling -- Reactor design; Chemical engineering -- Patents -- Periodicals; Chemical engineering -- Periodicals; Chemical industry -- Periodicals; Chemistry, Technical -- Periodicals; 660.05
• DOI: 10.1002/cite.201700160
• Languages: English
• ISSNs: 0009-286X

Abstract

Abstract: Microprocess engineering is an alternative approach to design reactors for CO2 methanation, which are used in power‐to‐gas applications. Microreactors offer advantages, e.g., in terms of heat removal. In the present work, design criteria evolved from transport phenomena are applied to derive preliminary reactor dimensions. The developed 1D model is used for parametric studies and reveals heat transport as limiting factor. More detailed 3D models confirm the results and demonstrate the effect of the metal matrix on heat transport. For further optimization a multi‐stage reactor design is proposed. Abstract : A microprocess engineering approach is used to design a chemical reactor for the methanation of carbon dioxide. One‐ and three‐dimensional reactor models are developed. Results of both models are in good agreement, which allows parametric studies on the one‐dimensional model. Additionally, a design concept is proposed to minimize the necessary amount of catalyst and reactor volume.