Ultrafast carrier dynamics of conformally grown semi-polar (112̄2) GaN/InGaN multiple quantum well co-axial nanowires on m-axial GaN core nanowires. Issue 22 (29th May 2019)

• Record Type: Journal Article
• Authors: Johar, Muhammad Ali; Song, Hyun-Gyu; Waseem, Aadil; Kang, Jin-Ho; Ha, Jun-Seok; Cho, Yong-Hoon; Ryu, Sang-Wan
• Is Part Of: Nanoscale. Volume 11:Issue 22(2019)
• Page Start: 10932
• Page End: 10943
• Publication Date: 2019-05-29
• Subjects: Nanoscience -- Periodicals; Nanotechnology -- Periodicals; 620.505
• DOI: 10.1039/c9nr02823d
• Languages: English
• ISSNs: 2040-3364

Abstract

Abstract : The growth of semi-polar (112̄2) GaN/InGaN multiple-quantum-well (MQW) co-axial heterostructure shells around m-axial GaN core nanowires on a Si substrate using MOCVD is reported for the first time. Abstract : The growth of semi-polar (112̄2) GaN/InGaN multiple-quantum-well (MQW) co-axial heterostructure shells around m-axial GaN core nanowires on a Si substrate using MOCVD is reported for the first time. The core GaN nanowire and GaN/InGaN MQW shells are grown in a two-step growth sequence of vapor–liquid–solid and vapor–solid growth modes. The luminescence and carrier dynamics of GaN/InGaN MQW coaxial nanowires are studied by photoluminescence, cathodoluminescence, and low temperature time-resolved photoluminescence (TRPL). The emission is tuned from 430 nm to 590 nm by increasing the InGaN QW thickness. The non-single exponential decay measured by low-temperature TRPL was attributed to the indium fluctuations in the InGaN QW. The ultrafast radiative lifetime was measured from 14 ps to 26 ps with different emission wavelengths at a very high internal quantum efficiency up to 68%. An ultrafast carrier lifetime was assigned to the growth of the InGaN QW on semi-polar (112̄2) growth facet and the improved carrier collection efficiency due to the radial growth of the GaN/InGaN MQW shells. Such an ultrafast carrier dynamics of NWs provides a meaningful active medium for high speed optoelectronic applications.