Efficient photoassociation of ultracold cesium atoms with picosecond pulse laser. (18th August 2017)

• Record Type: Journal Article
• Authors: Hai, Yang; Hu, Xue-Jin; Li, Jing-Lun; Cong, Shu-Lin
• Is Part Of: Molecular physics. Volume 115:Number 15/16(2017)
• Page Start: 1984
• Page End: 1991
• Publication Date: 2017-08-18
• Subjects: Photoassociation -- Gaussian and shaped laser pulse -- ultracold Cs atom and Cs2 molecule; Molecules -- Periodicals; Chemistry, Physical and theoretical -- Periodicals; Molécules -- Périodiques; Chimie physique et théorique -- Périodiques; 539.6.05
• DOI: 10.1080/00268976.2017.1332786
• Languages: English
• ISSNs: 0026-8976

Abstract

ABSTRACT: We investigate theoretically the formation of ultracold Cs2 molecules via photoassociation (PA) with three kinds of pulses (the Gaussian pulse, the asymmetric shaped laser pulse SL1 with a large rising time and a small falling time and the asymmetric shaped laser pulse SL2 with a small rising time and a large falling time). For the three kinds of pulses, the final population on vibrational levels from v ′ = 120 to 175 of the excited state displays a regular oscillation change with pulse width and interaction strength, and a high PA efficiency can be achieved with optimised parameters. The PA efficiency in the excited state steered by the SL1-pulse (SL2-pulse) train with optimised parameters which is composed of four SL1 (SL2) pulses is 1.74 times as much as that by the single SL1 (SL2) pulse due to the population accumulation effect. Moreover, a dump laser is employed to transfer the excited molecules from the excited state to the vibrational level v ″ = 12 of the ground state to obtain stable molecules. Abstract :