PAH emissions from an African cookstove. Issue 3 (June 2019)

• Record Type: Journal Article
• Authors: Lea-Langton, A.R.; Spracklen, D.V.; Arnold, S.R.; Conibear, L.A.; Chan, J.; Mitchell, E.J.S.; Jones, J.M.; Williams, A.
• Is Part Of: Journal of the Energy Institute. Volume 92:Issue 3(2019)
• Page Start: 587
• Page End: 593
• Publication Date: 2019-06
• Subjects: Cookstove -- Firewood -- Charcoal -- Particulate emissions -- PAH; Power (Mechanics) -- Periodicals; Power resources -- Periodicals; Fuel -- Periodicals; 621.04205
• DOI: 10.1016/j.joei.2018.03.014
• Languages: English
• ISSNs: 1743-9671

Abstract

Abstract: Combustion of wood and other biomass is a significant contributor to poor air quality in many developing countries. Emissions of particulates and Polycyclic Aromatic Hydrocarbons (PAH) are a major health hazard, particularly in Africa where the use of domestic cookstoves has increased alongside population expansion. Because of economic factors firewood is commonly used in place of the more expensive charcoal; particularly in rural areas. This work conducts a study of PAH emissions from an African cookstove comparing the combustion of both charcoal and firewood. It is demonstrated that PAH and particulate emissions are much higher from the firewood compared to the charcoal. The difference in levels can be interpreted due to the importance of the pyrolysis reactions of the volatile components of wood in PAH formation, whereas these volatiles emissions are much smaller from charcoal. Analysis of the combustion phases (flaming, smouldering) is undertaken and a computer model has been developed to link the composition of the fuels to the emissions of the PAH and particulates. The modelled PAH levels are shown to follow a similar trend to the experimental results. Highlights: Emissions of PAH and particulate emissions from an African cookstove are measured. Both fine particulates and PAH were significantly higher for firewood compared to charcoal. A computer model has been developed to understand the main features of the PAH emissions. The modelled PAH levels follow a similar trend to the experimental results.