Alternating-current driven quantum-dot light-emitting diodes with high brightness. Issue 12 (12th March 2019)

• Record Type: Journal Article
• Authors: Xia, Fengtian; Sun, Xiao Wei; Chen, Shuming
• Is Part Of: Nanoscale. Volume 11:Issue 12(2019)
• Page Start: 5231
• Page End: 5239
• Publication Date: 2019-03-12
• Subjects: Nanoscience -- Periodicals; Nanotechnology -- Periodicals; 620.505
• DOI: 10.1039/c8nr10461a
• Languages: English
• ISSNs: 2040-3364

Abstract

Abstract : Highly bright alternating-current (AC) driven quantum-dot light-emitting diodes (QLEDs) are demonstrated based on a single dielectric layer structure. Abstract : Highly bright alternating-current (AC) driven quantum-dot light-emitting diodes (QLEDs) are demonstrated based on a single dielectric layer structure. The use of a single dielectric layer P(VDF-TrFE-CFE) enables the injection of electrons under AC driving, whereas holes are generated inside the devices by using MoO3 /TFB hole generating layers. The brightness of the device is greatly affected by the capacitance of the dielectric layer, the hole generating capability of MoO3 /TFB and the driving frequency of the bias. By optimizing the thicknesses of P(VDF-TrFE-CFE) and MoO3 and the driving frequency, an AC-driven QLED with a luminance of 65 760 cd m −2 is demonstrated, which is the highest value ever reported. To improve the efficiency, a tandem AC-driven QLED is further developed, which alternately emits light in the positive and the negative driving cycles. As a result, the tandem AC-driven QLED exhibits a higher luminance and a current efficiency of 50 750 cd m −2 and 5.1 cd A −1, which are 1.3-fold higher than those (39 200 cd m −2, 3.9 cd A −1 ) of a single AC-driven QLED at the same current density. The demonstrated highly bright QLEDs that are directly driven by AC electricity could therefore eliminate the use of a direct-current (DC) power converter and could provide a potential alternative to conventional DC-driven devices for displays and lighting application.