Indoor emission, dispersion and exposure of total particle-bound polycyclic aromatic hydrocarbons during cooking. (November 2015)

• Record Type: Journal Article
• Authors: Gao, Jun; Jian, Yating; Cao, Changsheng; Chen, Lei; Zhang, Xu
• Is Part Of: Atmospheric environment. Volume 120(2015)
• Page Start: 191
• Page End: 199
• Publication Date: 2015-11
• Subjects: PAH -- Cooking -- Exposure -- Emission rate -- CFD -- Ventilation; Air -- Pollution -- Periodicals; Air -- Pollution -- Meteorological aspects -- Periodicals; 551.51
• DOI: 10.1016/j.atmosenv.2015.08.030
• Languages: English
• ISSNs: 1352-2310

Abstract

Abstract: Cooking processes highly contribute to indoor polycyclic aromatic hydrocarbon (PAH) pollution. High molecular weight and potentially carcinogenic PAHs are generally found attached to small particles, i.e., particulate phase PAHs (PPAHs). Due to the fact that indoor particle dynamics have been clear, describing the indoor dynamics of cooking-generated PPAHs within a specific time span is possible. This paper attempted to quantify the dynamic emission rate, simultaneous spatial dispersion and individual exposure of PPAHs using a cooking source. Experiments were conducted in a real-scale kitchen chamber to elucidate the time-resolved emission and effect of edible oil temperature and mass. Numerical simulations based on indoor particle dynamics were performed to obtain the spatial dispersion and individual inhalation intake of PPAHs under different emission and ventilation conditions. The present work examined the preheating cooking stage, at which edible oil is heated up to beyond its smoke point. The dynamic emission rate peak point occurred much earlier than the oil heating temperature. The total PPAH emission ranged from 2258 to 6578 ng upon heating 40–85 g of edible oil. The overall intake fraction by an individual within a period of 10 min, including 3 min for heating and 7 min for natural cooling, was generally ∼1/10, 000. An important outcome of this work was that the overall intake fraction could be represented by multiplying the range hood escape efficiency by the inhalation-to-ventilation rate ratio, which would be no greater than the same ratio. The methodology and results of this work were extendible for the number-based assessment of PPAHs. This work is expected to help us understand the health risks due to inhalation exposure to cooking-generated PPAHs in the kitchen. Highlights: Time-resolved emission, dispersion and individual intake of PPAHs were performed. Peak emission rate occurred significantly before the temperature peak. PPAHs dispersion was predicted with one single representative diameter. Indoor intake fraction of cooking-generated PPAHs was at ∼1/1, 0000. Intake fraction was less than the inhalation-to-ventilation rate ratio.