A comparative study of 129I content in environmental standard materials IAEA-375, NIST SRM 4354 and NIST SRM 4357 by Thermal Ionization Mass Spectrometry and Accelerator Mass Spectrometry. (August 2017)

• Record Type: Journal Article
• Authors: Olson, John; Adamic, Mary; Snyder, Darin; Brookhart, Jacob; Hahn, Paula; Watrous, Matthew
• Is Part Of: Applied radiation and isotopes. Volume 126(2017:Aug.)
• Page Start: 54
• Page End: 57
• Publication Date: 2017-08
• Subjects: AMS Accelerator Mass Spectrometry -- INL Idaho National Laboratory -- TIMS Thermal Ionization Mass Spectrometry -- TMAH tetramethylammonium hydroxide -- ESA electrostatic analyzer; AMS -- TIMS -- Iodine -- 129I -- Standards; Radiology -- Periodicals; Radiation -- Industrial applications -- Periodicals; Nuclear chemistry -- Periodicals; Internet resource; Periodical; 660.298
• DOI: 10.1016/j.apradiso.2017.01.028
• Languages: English
• ISSNs: 0969-8043

Abstract

Abstract: Iodine environmental measurements have consistently been validated in the literature using the standard material IAEA-375, soil collected approximately 160 miles northeast of Chernobyl, which is currently the only soil/sediment material with a certified 129 I activity. IAEA-375 has not been available for purchase since approximately 2010. Two other standard materials that are available (NIST SRM 4354, freshwater lake sediment and NIST SRM 4357, ocean sediment) have certified activities for a variety of radionuclides but not for 129 I. This paper reports a comparison of TIMS and AMS data for all three standards. Highlights: Limited 129 I data is available for NIST SRM-4354 and NIST SRM-4357. Preparation of environmental samples for TIMS and AMS analysis is described. TIMS and AMS showed agreement for 129 I in the environmental standards.