Collection and spectral control of high-order harmonics generated with a 50 W high-repetition rate Ytterbium femtosecond laser system. (29th March 2016)

• Record Type: Journal Article
• Authors: Cabasse, A; Hazera, Ch; Quintard, L; Cormier, E; Petit, S; Constant, E
• Is Part Of: Journal of physics. Volume 49:Number 8(2016:Apr. 15)
• Publication Date: 2016-03-29
• Subjects: high order harmonics -- femtosecond laser -- high repetition rate -- XUV source; Atoms -- Periodicals; Molecules -- Periodicals; Optics -- Periodicals; Nuclear physics -- Periodicals; 539.6
• DOI: 10.1088/0953-4075/49/8/085601
• Languages: English
• ISSNs: 0953-4075

Abstract

Abstract: We generate high-order harmonics with a 50 W, Yb femtosecond fiber laser system operating at 100 kHz in a tight focusing configuration. We achieve a high photon flux even with pulses longer than 500 fs. We collect the diverging extreme ultraviolet (XUV) harmonic beam in a 35 mrad wide solid angle by using a spectrometer designed to handle the high thermal load under vacuum and refocus the XUV beam onto a detector where the beam is characterised or can alternatively be used for experiments. This setup is designed for a 50 eV XUV bandwidth and offers the possibility to perform XUV-IR pump probe experiments with both temporal and spectral resolution. The high-order harmonics were generated and optimized at 100 kHz by using several gas target geometries (a gas jet and a semi-infinite gas cell) and several gases (argon, krypton, xenon) that provide XUV beams with different characteristics. After the spectrometer and for high-order harmonic generation (HHG) in xenon, we detect more than 4 × 10 10 photons per second over four harmonics, that is a useful XUV power on target of 0.1 μ W. This corresponds to the emission of more than 1 μ W per harmonic at the source and we achieved a similar flux with both the semi-infinite cell and the jet. In addition, we observe a strong spectral selectivity when generating harmonics in a semi-infinite gas cell as few harmonics clearly dominate the neighbouring harmonics. We attribute this spectral selectivity to phase matching effects.