On the apparent yield stress in non-Brownian magnetorheological fluids. Issue 39 (21st September 2017)

• Record Type: Journal Article
• Authors: Vågberg, Daniel; Tighe, Brian P.
• Is Part Of: Soft matter. Volume 13:Issue 39(2017)
• Page Start: 7207
• Page End: 7221
• Publication Date: 2017-09-21
• Subjects: Soft condensed matter -- Periodicals; 530.413
• DOI: 10.1039/c7sm01204g
• Languages: English
• ISSNs: 1744-683X

Abstract

Abstract : The viscosity of magnetorheological (MR) fluids can be increased dramatically by applying a magnetic field. Some MR fluids display a clear yield stress, while others do not. Using computer simulations, we rationalize this non-universal behavior in terms of the viscous interactions between particles and the carrier fluid. Abstract : We use simulations to probe the flow properties of dense two-dimensional magnetorheological fluids. Prior results from both experiments and simulations report that the shear stress σ scales with strain rate  as σ ∼  1− Δ, with values of the exponent ranging between 2/3 < Δ ≤ 1. However it remains unclear what properties of the system select the value of Δ, and in particular under what conditions the system displays a yield stress ( Δ = 1). To address these questions, we perform simulations of a minimalistic model system in which particles interact via long ranged magnetic dipole forces, finite ranged elastic repulsion, and viscous damping. We find a surprising dependence of the apparent exponent Δ on the form of the viscous force law. For experimentally relevant values of the volume fraction ϕ and the dimensionless Mason number Mn (which quantifies the competition between viscous and magnetic stresses), models using a Stokes-like drag force show Δ ≈ 0.75 and no apparent yield stress. When dissipation occurs at the contact, however, a clear yield stress plateau is evident in the steady state flow curves. In either case, increasing ϕ towards the jamming transition suffices to induce a yield stress. We relate these qualitatively distinct flow curves to clustering mechanisms at the particle scale. For Stokes-like drag, the system builds up anisotropic, chain-like clusters as Mn tends to zero (vanishing strain rate and/or high field strength). For contact damping, by contrast, there is a second clustering mechanism due to inelastic collisions.