Upper tropospheric water vapour and its interaction with cirrus clouds as seen from IAGOS long-term routine in situ observations. (2nd June 2017)

• Record Type: Journal Article
• Authors: Petzold, Andreas; Krämer, Martina; Neis, Patrick; Rolf, Christian; Rohs, Susanne; Berkes, Florian; Smit, Herman G. J.; Gallagher, Martin; Beswick, Karl; Lloyd, Gary; Baumgardner, Darrel; Spichtinger, Peter; Nédélec, Philippe; Ebert, Volker; Buchholz, Bernhard; Riese, Martin; Wahner, Andreas
• Is Part Of: Faraday discussions. Volume 200(2017)
• Page Start: 229
• Page End: 249
• Publication Date: 2017-06-02
• Subjects: Chemistry -- Periodicals; Metallurgy -- Periodicals; Electrochemistry -- Periodicals; 540
• DOI: 10.1039/c7fd00006e
• Languages: English
• ISSNs: 1359-6640

Abstract

Abstract : IAGOS (In-service Aircraft for a Global Observing System) performs long-term routine in situ observations of atmospheric chemical composition (O3, CO, NO x, NO y, CO2, CH4 ), water vapour, aerosols, clouds, and temperature on a global scale by operating compact instruments on board of passenger aircraft. The unique characteristics of the IAGOS data set originate from the global scale sampling on air traffic routes with similar instrumentation such that the observations are truly comparable and well suited for atmospheric research on a statistical basis. Here, we present the analysis of 15 months of simultaneous observations of relative humidity with respect to ice (RHice ) and ice crystal number concentration in cirrus ( N ice ) from July 2014 to October 2015. The joint data set of 360 hours of RHice – N ice observations in the global upper troposphere and tropopause region is analysed with respect to the in-cloud distribution of RHice and related cirrus properties. The majority of the observed cirrus is thin with N ice < 0.1 cm −3 . The respective fractions of all cloud observations range from 90% over the mid-latitude North Atlantic Ocean and the Eurasian Continent to 67% over the subtropical and tropical Pacific Ocean. The in-cloud RHice distributions do not depend on the geographical region of sampling. Types of cirrus origin ( in situ origin, liquid origin) are inferred for different N ice regimes and geographical regions. Most importantly, we found that in-cloud RHice shows a strong correlation to N ice with slightly supersaturated dynamic equilibrium RHice associated with higher N ice values in stronger updrafts.