Spatial and temporal distributions of 134Cs and 137Cs derived from the TEPCO Fukushima Daiichi Nuclear Power Plant accident in the North Pacific Ocean by using optimal interpolation analysis. Issue 1 (11th December 2015)

• Record Type: Journal Article
• Authors: Inomata, Y.; Aoyama, M.; Tsubono, T.; Tsumune, D.; Hirose, K.
• Is Part Of: Environmental science. Volume 18:Issue 1(2016)
• Page Start: 126
• Page End: 136
• Publication Date: 2015-12-11
• Subjects: Environmental monitoring -- Periodicals; Biological monitoring -- Periodicals; Environmental chemistry -- Periodicals; 363.7363
• DOI: 10.1039/c5em00324e
• Languages: English
• ISSNs: 2050-7887

Abstract

Abstract : Optimal interpolation (OI) analysis was used to investigate the oceanic distributions of 134 Cs and 137 Cs released from the Tokyo Electric Power Company Fukushima Daiichi Nuclear Power Plant (FNPP1) accident. Abstract : Optimal interpolation (OI) analysis was used to investigate the oceanic distributions of 134 Cs and 137 Cs released from the Tokyo Electric Power Company Fukushima Daiichi Nuclear Power Plant (FNPP1) accident. From the end of March to early April 2011, extremely high activities were observed in the coastal surface seawater near the FNPP1. The high activities spread to a region near 165°E in the western North Pacific Ocean, with a latitudinal center of 40°N. Atmospheric deposition also caused high activities in the region between 180° and 130°W in the North Pacific Ocean. The inventory of FNPP1-released 134 Cs in the North Pacific Ocean was estimated to be 15.3 ± 2.6 PBq. About half of this activity (8.4 ± 2.6 PBq) was found in the coastal region near the FNPP1. After 6 April 2011, when major direct releases ceased, the FNPP1-released 134 Cs in the coastal region decreased exponentially with an apparent half-time of about 4.2 ± 0.5 days and declined to about 2 ± 0.4 PBq by the middle of May 2011. Taking into account that the 134 Cs/ 137 Cs activity ratio was about 1 just after release and was extremely uniform during the first month after the accident, the amount of 137 Cs released by the FNPP1 accident increased the North Pacific inventory of 137 Cs due to bomb testing during the 1950s and early 1960s by 20%.