Effects of meteorological conditions on sulfur dioxide air pollution in the North China plain during winters of 2006–2015. (December 2016)

• Record Type: Journal Article
• Authors: Calkins, Chase; Ge, Cui; Wang, Jun; Anderson, Mark; Yang, Kai
• Is Part Of: Atmospheric environment. Volume 147(2016)
• Page Start: 296
• Page End: 309
• Publication Date: 2016-12
• Subjects: SO2 -- Air pollution meteorology and climatology -- OMI -- GEOS-Chem; Air -- Pollution -- Periodicals; Air -- Pollution -- Meteorological aspects -- Periodicals; 551.51
• DOI: 10.1016/j.atmosenv.2016.10.005
• Languages: English
• ISSNs: 1352-2310

Abstract

Abstract: The last decade has seen frequent occurrences of severe air pollution episodes of high loading in SO2 during winters in the North China Plain (NCP). Using satellite data from the Ozone Monitoring Instrument (OMI), chemistry transport model (GEOS-Chem) simulations, and National Center for Environmental Predication (NCEP) meteorological reanalysis, this study examines meteorological and synoptic conditions associated with air pollution episodes during 2006–2015 winters. OMI-based SO2 data suggest a large decrease (∼30% in area average) of SO2 emissions since 2010. Statistical analysis shows that meteorological conditions associated with the top 10% of OMI-based high SO2 days are found on average to be controlled by high pressure systems with 2 m s −1 lower wind speeds, slightly warmer, 1–2 °C, temperatures and 10–20% higher relative humidities from the surface to 850 hPa. Numerical experiments with GOES-Chem nested grid simulations at 0.5° × 0.667° resolution are conducted for winters of 2009 as a control year, and 2012 and 2013 as years for sensitivity analysis. The experiments reveal that year-to-year change of winter columnar SO2 amounts and distributions in first order are linearly proportional to the change in SO2 emissions, regardless of the differences in meteorological conditions. In contrast, the surface SO2 amounts and distributions exhibit highly non-linear relationships with respect to the emissions and stronger dependence on the meteorological conditions. Longer data records of atmospheric SO2 from space combined with meteorological reanalysis are needed to further study the meteorological variations in air pollution events and the air pollution climatology in the context of climate change. Highlights: Meteorological conditions with OMI-based high SO2 days in China are studied. Climatological anomaly of meteorological variables in high SO2 days are quantified. Year-to-year winter change of columnar SO2 distribution is mostly due to SO2 emission. Surface SO2 distribution has stronger dependence on meteorology than columnar SO2. Columnar SO2 climatology is not representative to surface SO2 climatology.