Two‐Dimensional Supramolecular Electron Spin Arrays. (22nd January 2013) - Wäckerlin, Christian
Abstract A bottom‐up approach is introduced to fabricate two‐dimensional self‐assembled layers of molecular spin‐systems containing Mn and Fe ions arranged in a chessboard lattice. We demonstrate that the Mn and Fe spin states can be reversibly operated by their selective response to coordination/decoordination of volatile ligands like ammonia (NH3).