Persistent Photoconductivity in 2D Electron Gases at Different Oxide Interfaces. Issue 11 (19th August 2013)

• Record Type: Journal Article
• Authors: Di Gennaro, Emiliano; di Uccio, Umberto Scotti; Aruta, Carmela; Cantoni, Claudia; Gadaleta, Alessandro; Lupini, Andrew R.; Maccariello, Davide; Marré, Daniele; Pallecchi, Ilaria; Paparo, Domenico; Perna, Paolo; Riaz, Muhammad; Granozio, Fabio Miletto
• Is Part Of: Advanced optical materials. Volume 1:Issue 11(2013:Nov.)
• Page Start: 834
• Page End: 843
• Publication Date: 2013-08-19
• Subjects: Optical materials -- Periodicals; Photonics -- Periodicals; 620.11295
• DOI: 10.1002/adom.201300150
• Languages: English
• ISSNs: 2195-1071

Abstract

<abstract abstract-type="main" xml:lang="en"> <title> <x xml:space="preserve">Abstract</x> </title> <p>The transport characterization in the dark and under light irradiation of three different interfaces—LaAlO<sub>3</sub>/SrTiO<sub>3</sub>, LaGaO<sub>3</sub>/SrTiO<sub>3</sub>, and the novel NdGaO<sub>3</sub>/SrTiO<sub>3</sub> heterostructure—is reported. All of them share a perovskite structure, an insulating nature of the single building blocks, a polar/non‐polar character, and a critical thickness of four unit cells for the onset of conductivity. The interface structure and charge confinement in NdGaO<sub>3</sub>/SrTiO<sub>3</sub> are probed by atomic‐scale‐resolved electron energy loss spectroscopy showing that, similarly to LaAlO<sub>3</sub>/SrTiO<sub>3</sub>, extra electronic charge confined in a sheet of about 1.5 nm in thickness is present at the NdGaO<sub>3</sub>/SrTiO<sub>3</sub> interface. Electric transport measurements performed in the dark and under radiation show remarkable similarities and provide evidence that the persistent perturbation induced by light is an intrinsic peculiar property of the three investigated oxide‐based polar/non‐polar interfaces. This sets a framework for understanding the previous contrasting results found in the literature about photoconductivity in LaAlO<sub>3</sub>/SrTiO<sub>3</sub> and highlights the connection between the origin of persistent photoconductivity and the origin of conductivity itself. An improved understanding of the photoinduced metastable electron–hole pairs might allow light to be shed directly on the complex physics of this system and on the recently proposed perspectives of oxide interfaces for solar energy conversion.</p> </abstract>